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Nadesico is fun in the same sort of wacky black heaven way. What better way to follow up a galactic concert by Black Heaven but a talent show on the UN Spacey Nadesico?
The Knight Sabres are a vigilante team in a futuristic world. 2033 isn't as modern as the more recent BGC 2040 but if you like robotically agumented soldiers it's worth checking out.
Eva is kind of like Lain, but with mechs thrown into the equation as well. If you liked Lain, you might enjoy Eva.
If you liked the drama in Sign check out Haibane Renmei. A very touching story
Tenchi Muyo is another fun romantic comedy.
Gasaraki is another Mech based anime. Mostly ground combat and no flying but it's defenatly worth a look if you like the tactical side of a VF series in combat.
If you take all of Love Hinas obsurdities and crazy situations (Mechatama!!!) condense them into six eppisodes then multiply them by three you kind of get a feel for what FLCL is like.
Another serious series. There are forces at work here that we dont know much about.
Love Hina is a much tamer love story that occationally has seens that are obsurd enough to be like FLCL, including giant turtle robots. Imagine the crazyness of FLCL stretched to fit over 32 eppisodes instead of condensed into six.
WHR folows a similar format as Noir. All of the characters get caught up in something much larger than they had ever imagined.
Yet more high school antics! AD is more on the cutsie side of anime than GTO, but the teachers are no less crazy. :)
Hellsing is another series that takes a darker more serious aproach. STNs mission is very similar to the Hellsing Organisations.
Boogiepop Phantom is another weird and trippy series. The story isn't as linearly defined and it touches on interesting psychological situations, just like in Lain.
Another kind of cyberpunk story. Cybernetic soldiers in a digital future world.
Ranma 1/2 is another lovers in denial story. Expect more misunderstandings and physical punishment!
Welcome to the world of professional female assasins. Another gun toting series.
HL is a lot like Love Hina without the love interest. Throw five women with vastly different personalities into the same house with poor Chitose and watch the sparks fly as they each try to become the "best mother".
Another mech series where things are more complicated than they seem.
GTO is another anime involving school antics. It's less cutsie and more reckless and wild than Azumanga. If you liked AD then you must check it out!