If you're looking for anime similar to Angelique ~When the Heart Awakens~, you might like these titles. All recommendations are made by Anime-Planet users like you!
Once there lived an eccentric author called Drosselmeyer who wrote grand tragedies - one of them was the tale of a prince who sealed away an evil raven by breaking his own heart into tiny pieces. However, before the story could be completed, the author died and the tale took on a life of its own. Now, in a town where fiction and reality meet, the story continues on its tragic course with Ahiru, a duck who transforms into the beautiful Princess Tutu in order to restore the prince's heart. But will Ahiru's act of love be enough to defy the story's terrible destiny and lead to a happy ending?
Princess Tutu shares that episodic format with Angelique where a girl must collect fragments in order to heal a whole, along the way having numerous adventures. However, anyone thinking Angelique is entertaining should immediately proceed to watch Princess Tutu! It's an outstanding anime that actually creates a fresh, funny, and eccentric story around shoujo cliches like bishies, ballet, fairytales, cutesie animation etc. You will not be disappointed, trust me.
While reading "The Universe of the Four Gods", best friends Miaka and Yui are mysteriously transported into a strange world full of magic and unfamiliar faces. As if their arrival was determined by fate, Miaka is revered as the Priestess of Suzaku, the savior of their warring country, who was destined to arrived in a flash of light, from a land far away. Betrayal, love, and heartache accompany this fantasy-filled tale of friendships torn apart, and hope that never fades.
Fushigi Yugi: The mysterious play has the same reverse harem feel. Hot guys with one girl that must save someone or something because they are destined. Fushigi Yugi is about two girls but only one is the main character that is sent into a alternate time where it was the era of men with ponytails and long hair. Where Angelique movie is sent to a time where time stops altogether. Both are long and have alot of OVAs however the characters are liked some of the time.
After the events of the Onikirimaru incident, Tamaki thinks that her days of trouble are finally behind her. But when Logos reappears with a deadly plot, one of the five Guardians is revealed to be a traitor! With the people closest to her now in question, Tamaki will have to decide who she can truly trust if she wants to stop Logos for good. The truth behind the Tamayori Princess will finally be revealed as Tamaki battles evil once again!
This series (including both the sequel to this one and the spin off Neo Angelique) is very similar in the way that the main protagonist is a girl who has special powers and she is protected by the male characters. The female protagonist has the same attitude as the female protagonist in Hiiro no Kakera in that she is always optimistic and generous. I liked these anime because they really do a good job of developing the main characters, despite the fact that there are so many of them. Compared to Hiiro no Kakera, the Angelique series is much lighter, but I like to think the lightness of this one has a certain charm.